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Being a Synchro and banish-centered Psychic archetype, "PSY-Frame" has great synergy with general Psychic support such as "Esper Girl", "Psychic Feel Zone", "Psychic Path", "Bright Future" and "Past Image", for example

A card can have two expend costs, like Muerra, Trash Tactician having expend 4 and expend 8 on it, but both of those only trigger the first time you spend that amount of mana

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What sets this card apart is that while Azula is attacking, each spell you cast is copied, so Azula is an excellent storm enabler when you can copy rituals, cantrips, Frantic Searches, and the like